I would actually suggest the Max1674 or something with similar specs. The ICs you linked to had cutoff Vin of 2.7V. This would work better with 3 cells, since with 2 cells, you would very quickly reach 2.7V and still not have tapped even half the available power in the cells. The 1674 cuts off at 0.7V, so your cells would be properly used up.
Also, I have an idiosyncracy. I prefer using voltage regulation when running 5mm LED arrays. This is in the event that if one of the LEDs malfunctions, the circuit automatically compensates and reduces the current flowing, though the voltage remains constant. A current regulated circuit would continue to provide the same amount of current which must now be distributed among fewer LEDs. Sometimes, the increase in power-per-LED may be sufficient to blow out the other LEDs.
Best of luck with the Max1674 though. It is surface mounted and rather difficult to solder.